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Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1091-x

摘要：

Ratio of turbidity and TSS (Tur/TSS) was used to characterize PSD of stormwater particles.

Pb and Zn preferred to accumulate in finer RDS, while Cu, Cr and Ni in coarser RDS.

HMs pollution in stormwater particles increased linearly with Tur/TSS.

Dissolvability of HMs and PSD variations contribute to the differences between RDS and stormwater.

关键词： Road-deposited sediment     Stormwater runoff     Heavy metal     Particle size     Pollution variation    

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ZnFe2O4 deposited on BiOCl with exposed (001) and (010) facets for photocatalytic

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

《化学科学与工程前沿（英文）》 2017年 第11卷 第2期   页码 197-204 doi: 10.1007/s11705-016-1606-y

摘要： ZnFe O -BiOCl composites were prepared by both hydrothermal and direct precipitation processes and the structures and properties of the samples were characterized by various instrumental techniques. The samples were then used as catalysts for the photocatalytic reduction of CO in cyclohexanol under ultraviolet irradiation to give cyclohexanone (CH) and cyclohexyl formate (CF). The photocatalytic CO reduction activities over the hydrothermally prepared ZnFe O -BiOCl composites were higher than those over the directly-precipitated composites. This is because compared to the direct-precipitation sample, the ZnFe O nanoparticles in the hydrothermal sample were smaller and more uniformly distributed on the surface of BiOCl and so more heterojunctions were formed. Higher CF and CH yields were obtained for the pure BiOCl and BiOCl composite samples with more exposed (001) facets than for the samples with more exposed (010) facets. This is due to the higher density of oxygen atoms in the exposed (001) facets, which creates more oxygen vacancies, and thereby improves the separation efficiency of the electron-hole pairs. More importantly, irradiation of the (001) facets with ultraviolet light produces photo-generated electrons which is helpful for the reduction of CO to ·CO . The mechanism for the photocatalytic reduction of CO in cyclohexanol over ZnFe O -BiOCl composites with exposed (001) facets involves electron transfer and carbon radical formation.

关键词： reduction of CO2     cyclohexanol     ZnFe2O4 deposited BiOCl     facet     composite photocatalyst    

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Effects of previous drying of sediment on root functional traits and rhizoperformance of emerged macrophytes

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1427-1

摘要：

• Sediment desiccation alters morphological characteristics of aquatic sediment.

关键词： Fibrous-root macrophytes     Thick-root macrophytes     Nutrients removal     Wet sediment     Dried-rewetted sediment    

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Growth and properties analysis of metal-organic chemical vapor deposited MgZnO films on -AlO substrates

SHI Zengliang, LIU Dali, YAN Xiaolong, GAO Zhongmin, BAI Shiying

《机械工程前沿（英文）》 2008年 第3卷 第3期   页码 261-264 doi: 10.1007/s11465-008-0036-z

摘要： MgZnO (0 < ? 0.12) thin films with the wurtzite structure have been successfully grown on -AlO substrates by metal-organic chemical vapor deposition (MOCVD). X-ray photoelectron spectroscopy (XPS), X-ray diffraction (XRD), photoluminescence (PL) spectrometry, and transmission measurements are performed to study the characteristics of MgZnO thin films. Results show that with increasing Mg content, the diffraction peak of MgZnO thin films shifts towards a higher diffraction angle (the biggest shift is 0.22°), and the full width at half maximum (FWHM) of the diffraction peak is broadened. Meanwhile, a blue-shift occurs at the near-band-edge (NBE) emission peak and the largest blue-shift of the band gap of the MgZnO films is 113 meV with Mg content = 0.12. Therefore, the energy band gap of the MgZnO films is determined by Mg content in the thin films and the energy band gap increases with an increase of Mg content.

关键词： increase     photoelectron spectroscopy     transmission     wurtzite structure     MgZnO    

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Diversity and vertical distributions of sediment bacteria in an urban river contaminated by nutrients

Xunan YANG, Shan HUANG, Qunhe WU, Renduo ZHANG, Guangli LIU

《环境科学与工程前沿（英文）》 2013年 第7卷 第6期   页码 851-859 doi: 10.1007/s11783-013-0569-1

摘要： The aim of this study was to investigate the benthic bacterial communities in different depths of an urban river sediment accumulated with high concentrations of nutrients and metals. Vertical distributions of bacterial operational taxonomic units (OTUs) and chemical parameters (nutrients: , , dissolved organic carbon, and acid volatile sulfur; metals: Fe, Zn, and Cu) were characterized in 30 cm sediment cores. The bacterial OTUs were measured using the terminal restriction fragment length polymorphism analysis. Biodiversity indexes and multivariate statistical analyses were used to characterize the spatial distributions of microbial diversity in response to the environmental parameters. Results showed that concentrations of the nutrients and metals in this river sediment were higher than those in similar studies. Furthermore, high microbial richness and diversity appeared in the sediment. The diversity did not vary obviously in the whole sediment profile. The change of the diversity indexes and the affiliations of the OTUs showed that the top layer had different bacterial community structure from deeper layers due to the hydrological disturbance and redox change in the surface sediment. The dominant bacterial OTUs ubiquitously existed in the deeper sediment layers (5–27 cm) corresponding to the distributions of the nutrients and metals. With much higher diversity than the dominant OTUs, the minor bacterial assemblages varied with depths, which might be affected by the sedimentation process and the environmental competition pressure.

关键词： heavy metals     nutrients     sediment profile     terminal restriction fragment length polymorphism    

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Microbial responses to the use of NaClO in sediment treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第2期 doi: 10.1007/s11783-021-1451-1

摘要：

• Chlorine addition enhanced the release of TOC, TN from the sediment.

关键词： Sediment chlorination     Substance mobility     Microbial response     Community composition     Function    

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黄土高原生态重建的水沙效应研究 Article

孙彭成, 吴一平, 杨志峰, Bellie Sivakumar, 邱临静, 刘曙光, 蔡宴朋

《工程（英文）》 2019年 第5卷 第5期   页码 855-864 doi: 10.1016/j.eng.2019.07.014

摘要：

黄土高原是全球土壤侵蚀最为严重的区域之一，也是黄河泥沙的主要来源。自20世纪50年代大规模水土保持措施实施以来，该地区入黄泥沙量持续减少,流域内泥沙来源与输移机制变得更为复杂，对水土保持措施作用下的河流输沙及变异特征的研究一直是学界关注的重点。本文以水土保持治理成效最为显著的黄土丘陵沟壑区的典型区域为研究对象，采用近50年的水沙观测数据，分析水土保持作用下流域水沙关系演变。结果表明，水土保持措施的实施引发流域水沙关系的显著变化，具体表现为幂指数水沙关系中系数的减小和指数的增加，且前阶段指数增加缓慢而后期增加剧烈。幂指数的增加表征新的更加陡峭的水沙关系曲线，意味着流域年际输沙变异程度或将增强。此外，新旧水沙关系曲线存在一个临界交点，在新的水沙关系条件下，低于临界流量的径流将输移更少的泥沙，这也是该地区泥沙输移新的主导状态；然而，大于临界流量的极端径流也有可能引发更强的泥沙输移。因此，本文认为黄土高原的低泥沙输移未必是一种新常态，极端洪水条件下仍有强输沙的可能性而需增强防范。

关键词： 流域水沙关系     生态恢复     黄土丘陵沟壑区     泥沙输移     水沙关系参数    

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Characteristics and application of road absorbing solar energy

Zhihua ZHOU, Shan HU, Xiaoyan ZHANG, Jian ZUO

《能源前沿（英文）》 2013年 第7卷 第4期   页码 525-534 doi: 10.1007/s11708-013-0278-2

摘要： If the heat of road surface can be stored in summer, the road surface temperature will be decreased to prevent permanent deformation of pavement. Besides, if the heat stored is released, it can supply heat for buildings or raise the road surface temperature for snow melting in winter. A road-solar energy system was built in this study, and the heat transfer mechanism and effect of the system were analyzed according to the monitored solar radiant heat, the solar energy absorbed by road and the heat stored by soil. The results showed that the road surface temperature was mainly affected by solar radiation, but the effect is hysteretic in nature. The temperature of the solar road surface was 3°C–6°C lower than that of the ordinary road surface. The temperature of the solar road along the vertical direction was 2°C–5°C lower than that of the ordinary road. The temperature difference increased as the distance to the heat transfer tubes decreased. The average solar collector efficiency of the system was 14.4%, and the average solar absorptivity of road surface was 36%.

关键词： solar energy     road-solar energy system     road surface temperature     solar absorptivity of road surface     solar collector efficiency of system    

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Red soil for sediment capping to control the internal nutrient release under flow conditions

Lei Xia, Guo Liu, Chunmei Chen, Meiyan Wen, Yangyang Gao

《环境科学与工程前沿（英文）》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0886-2

摘要： The inhibition of sediment nitrogen (N) and phosphorus (P) release seems necessary. Red soil (RS) was firstly used as sediment capping material under flow conditions. RS capping can effectively reduce the N and P release from sediment. Nitrogen (N) and phosphorus (P) released from the sediment to the surface water is a major source of water quality impairment. Therefore, inhibiting sediment nutrient release seems necessary. In this study, red soil (RS) was employed to control the nutrients released from a black-odorous river sediment under flow conditions. The N and P that were released were effectively controlled by RS capping. Continuous-flow incubations showed that the reduction efficiencies of total N (TN), ammonium (NH -N), total P (TP) and soluble reactive P (SRP) of the overlying water by RS capping were 77%, 63%, 77% and 92%, respectively, and nitrification and denitrification occurred concurrently in the RS system. An increase in the water velocity coincided with a decrease in the nutrient release rate as a result of intensive water aeration.

关键词： Sediment     Red soil capping     Flow conditions     Nitrogen     Phosphorus    

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Four kinds of capping materials for controlling phosphorus and nitrogen release from contaminated sediment

《环境科学与工程前沿（英文）》 2022年 第16卷 第3期 doi: 10.1007/s11783-021-1463-x

摘要：

• Lanthanum modified bentonite (LMB) can effectively absorb phosphorus (P).

关键词： Sediment     Eutrophication     Thin-layer capping     Phosphorus     Nitrogen     Aluminum-based P-inactivation agent    

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Development and road performance of clear asphalt with high transparency and adhesion

《结构与土木工程前沿（英文）》 2023年 第17卷 第2期   页码 238-255 doi: 10.1007/s11709-022-0898-x

摘要： Clear asphalt (CA) currently used in light-colored asphalt mixtures (LCAM) exhibits poor transparency and adhesion. Therefore, a highly transparent CA (HCA) modified using a silane coupling agent (KH550) was prepared. Furthermore, LCAM was prepared by mixing CA and limestone aggregates. The properties of the HCA and ordinary CA (OCA) were characterized using conventional asphalt tests, optical tests, pull-off tests, ultraviolet aging tests, dynamic shear rheometry, Fourier-transform infrared spectroscopy, differential scanning calorimetry, and scanning electron microscopy. Whereas Marshall, moisture resistance, wheel tracking, trabecular bending, and British pendulum tests were employed for the LCAM. The transmittance and spectral reflectance of the HCA were 123.30 and 3.74 times greater than those of the OCA, respectively. The complex modulus and viscosity-aging index of the HCA were 48% and 53% less than those of the OCA, respectively. After modification with KH550, the Marshall stability ratio, tensile strength ratio, and flexural strain of the HCA-prepared LCAM increased by 12.92%, 25.06%, and 23.90%, respectively. However, the rutting resistance of the HCA-prepared LCAM was 14.3% less than that of the OCA-prepared LCAM. The comprehensive performances of the HCA and HCA-prepared LCAM were 49.2% and 10.3% greater than those of the OCA and OCA-prepared LCAM, respectively, indicating a high application value in the future.

关键词： light-colored asphalt pavement     orthogonal test     road performance     spectral reflectance     silane-coupling agent    

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Characterization of interaction between different adsorbents and copper by simulation experiments using sediment-extracted

Yan ZHANG,Yuan ZHANG,Tao YU

《环境科学与工程前沿（英文）》 2014年 第8卷 第4期   页码 510-518 doi: 10.1007/s11783-013-0588-y

摘要： The complex capacity of different types of organic matters (OMs) for Cu was quantitatively studied by simulation experiments using different adsorbents prepared from the sediment in Taihu Lake. The free Cu was measured with ion selective electrode (ISE) and complex capacity was calculated using a conditional formation constant model. The result indicated that the complex capacity was 0.048 mmol·g , 0.009 and 0.005 mmol·g for raw sediment, sediment without DOM, sediment without insoluble organic matters but with DOM and sediment without OM. Insoluble organic matter played a major role in the sorption of Cu in sediment and it can adsorb most Cu from water column. In the solution, Cu mainly existed as a complex with DOM and the DOM-Cu complexation capacity was 327.87 mg·g . The change of TOC and pH indicated ion-exchange in the interaction between free Cu and DOM. When the Cu concentration in the experiment reached the complex capacity of DOM, precipitation was the major mechanism to remove Cu from water phase, which was observed from UV absorbance change of DOM, that is, its aromaticity increased while molecular weight decreased. The desorption result indicated that DOM was more capable of desorbing Cu from adsorbents without OM than adsorbent with OM. The desorbed quantity with DOM was 1.65, 1.78 and 2.25 times higher than that with water for adsorbents without OM, raw adsorbents (sediment) and adsorbents without DOM.

关键词： interaction     dissolved organic matters     sediment     sorption     desorption     Taihu Lake    

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Special issue: Management of road and railway traffic and transportation engineering

Yongfu SUN, Ziyou GAO

《工程管理前沿（英文）》 2017年 第4卷 第4期   页码 385-387 doi: 10.15302/J-FEM-2017110

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Effects of different sediment fractions on sorption of galaxolide

Lixia JIN, Mengchang HE, Jinghuan ZHANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第1期   页码 59-65 doi: 10.1007/s11783-010-0259-1

摘要： Sorption isotherms of galaxolide (HHCB) of different fractions from two sediments with different mineral and organic carbon contents were determined to compare HHCB sorption behavior and contribution to the total sorption. The HHCB sorption isotherms that used the batch equilibration method were studied on different sediments of different fractions. The sorption isotherms of 600°C heating fractions were detailed using the linear model, while the other fractions were nonlinear and fitted well with the Freundlich model. The dissolved organic carbon (DOC) removed, NaOH extracted, and 375°C heating fractions showed more nonlinear sorption than the original sediments, which suggested more heterogeneous sorption sites in these fractions. Compared to the original sediments, the 375°C heating fractions had higher carbon-normalized distribution coefficient ( ) values, indicating a higher sorption affinity for HHCB. Among the different sediment fractions, the contribution of the 600°C heating fractions to the overall sorption were the lowest (<20%), while the 375°C heating fractions were the highest (up to 85%).

关键词： galaxolide (HHCB)     sorption     organic carbon     sediment     carbon-normalized distribution coefficient (Koc)    

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新形势下黄河水沙调控策略研究

胡春宏,张双虎,张晓明

《中国工程科学》 2022年 第24卷 第1期   页码 122-130 doi: 10.15302/J-SSCAE-2022.01.013

摘要：

黄河水沙调控对保障黄河长久安澜至关重要。近几十年来，受自然因素和水土保持等人类活动的双重影响，黄河来水来沙量持续发生变化，水资源量略有减少、来沙量锐减，为此，科学研判未来黄河来水来沙量是制定水沙调控策略最基础、最关键的科学问题。本文分析了1919—2020 年百年尺度下的黄河来水来沙量的演变情况，并预测了未来50 年的黄河来水来沙量；系统总结了目前黄河水沙调控面临的主要问题，即黄河上游河道淤积萎缩、黄河下游滩区治理策略与高质量发展要求不适应、黄土高原水土流失治理区域不均衡等。在此基础上，提出了新水沙条件下的黄河水沙调控策略建议，一是以黄河上游黑山峡河段开发和古贤水利枢纽建设为重点，完善水沙调控体系；二是黄河下游滩区分区治理、改造河道并释放部分滩区，实现滩区防洪运用与高质量发展的协同；三是科学开展黄土高原分区分类水土保持措施，调整黄土高原治理格局，协同推进生态保护和乡村振兴。

关键词： 黄河     新水沙条件     水沙调控     水利枢纽     分区治理     生态保护    

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标题 作者 时间 类型 操作

Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

期刊论文

ZnFe2O4 deposited on BiOCl with exposed (001) and (010) facets for photocatalytic

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

期刊论文

Effects of previous drying of sediment on root functional traits and rhizoperformance of emerged macrophytes

期刊论文

Growth and properties analysis of metal-organic chemical vapor deposited MgZnO films on -AlO substrates

SHI Zengliang, LIU Dali, YAN Xiaolong, GAO Zhongmin, BAI Shiying

期刊论文

Diversity and vertical distributions of sediment bacteria in an urban river contaminated by nutrients

Xunan YANG, Shan HUANG, Qunhe WU, Renduo ZHANG, Guangli LIU

期刊论文

Microbial responses to the use of NaClO in sediment treatment

期刊论文

黄土高原生态重建的水沙效应研究

孙彭成, 吴一平, 杨志峰, Bellie Sivakumar, 邱临静, 刘曙光, 蔡宴朋

期刊论文

Characteristics and application of road absorbing solar energy

Zhihua ZHOU, Shan HU, Xiaoyan ZHANG, Jian ZUO

期刊论文

Red soil for sediment capping to control the internal nutrient release under flow conditions

Lei Xia, Guo Liu, Chunmei Chen, Meiyan Wen, Yangyang Gao

期刊论文

Four kinds of capping materials for controlling phosphorus and nitrogen release from contaminated sediment

期刊论文

Development and road performance of clear asphalt with high transparency and adhesion

期刊论文

Characterization of interaction between different adsorbents and copper by simulation experiments using sediment-extracted

Yan ZHANG,Yuan ZHANG,Tao YU

期刊论文

Special issue: Management of road and railway traffic and transportation engineering

Yongfu SUN, Ziyou GAO

期刊论文

Effects of different sediment fractions on sorption of galaxolide

Lixia JIN, Mengchang HE, Jinghuan ZHANG

期刊论文

新形势下黄河水沙调控策略研究

胡春宏,张双虎,张晓明

期刊论文